measurement-coherence-decay-gamnas-using-femtosecond-four-wave

Measurement of Coherence Decay in GaMnAs Using Femtosecond Four-wave Mixing

The application of femtosecond four-wave mixing to the study of fundamental properties of diluted magnetic semiconductors ((s,p)-d hybridization, ...

University of Notre Dame

According to quantum mechanics, a many-particle system is allowed to exhibit non-local behaviour, in that measurements performed on one of the particles can affect a second one that is far away. These so-called entangled states are crucial for the implementation of most quantum information protocols and, in particular, gates for quantum computation. Here we use ultrafast optical pulses and coherent techniques to create and control spin-entangled states in an ensemble of non-interacting electrons bound to donors (at least three) and at least two Mn2+ ions in a CdTe quantum well. Our method, relying on the exchange interaction between localized excitons and paramagnetic impurities, can in principle be applied to entangle an arbitrarily large number of spins.

Optically induced multispin entanglement in a semiconductor quantum well.

The photoluminescence of colloidal Mn2+-doped CdSe nanocrystals has been studied as a function of nanocrystal diameter. These nanocrystals are shown to be unique among colloidal doped semiconductor nanocrystals reported to date in that quantum confinement allows tuning of the CdSe bandgap energy across the Mn2+ excited-state energies. At small diameters, the nanocrystal photoluminescence is dominated by Mn 2+ emission. At large diameters, CdSe excitonic photoluminescence dominates. The latter scenario has allowed spin-polarized excitonic photoluminescence to be observed in colloidal doped semiconductor nanocrystals for the first time.

Spin-polarizable excitonic luminescence in colloidal Mn2+-doped CdSe quantum dots.

Thin epitaxial films of the diluted magnetic semiconductor (DMS) GaMnAs have been studied by low energy muon spin rotation and relaxation (LE-microSR) as well as by transport and magnetization measurement techniques. LE-microSR allows measurements of the distribution of magnetic field on the nanometer scale inaccessible to traditional macroscopic techniques. The spatial inhomogeneity of the magnetic field is resolved: although homogeneous above Tc, below Tc the DMS consists of ferromagnetic and paramagnetic regions of comparable volumes. In the ferromagnetic regions the local field inhomogeneity amounts to 0.03 T.

Spatially resolved inhomogeneous ferromagnetism in (Ga,Mn)as diluted magnetic semiconductors: a microscopic study by muon spin relaxation.

Doping of semiconductor nanocrystals by transition-metal ions has attracted tremendous attention owing to their nanoscale spintronic applications. Such doping is, however, difficult to achieve in low-dimensional strongly quantum confined nanostructures by conventional growth procedures. Here we demonstrate that the incorporation of manganese ions up to 10% into CdSe quantum nanoribbons can be readily achieved by a nucleation-controlled doping process. The cation-exchange reaction of (CdSe)(13) clusters with Mn(2+) ions governs the Mn(2+) incorporation during the nucleation stage. This highly efficient Mn(2+) doping of the CdSe quantum nanoribbons results in giant exciton Zeeman splitting with an effective g-factor of approximately 600, the largest value seen so far in diluted magnetic semiconductor nanocrystals. Furthermore, the sign of the s-d exchange is inverted to negative owing to the exceptionally strong quantum confinement in our nanoribbons. The nucleation-controlled doping strategy demonstrated here thus opens the possibility of doping various strongly quantum confined nanocrystals for diverse applications.

Article	Year
Optically induced multispin entanglement in a semiconductor quantum well. Nature materials\| PubMed ID: 12612675	2003
Spin-polarizable excitonic luminescence in colloidal Mn2+-doped CdSe quantum dots. Nano letters\| PubMed ID: 18331001	2008
Spatially resolved inhomogeneous ferromagnetism in (Ga,Mn)as diluted magnetic semiconductors: a microscopic study by muon spin relaxation. Physical review letters\| PubMed ID: 18764221	2008
Giant Zeeman splitting in nucleation-controlled doped CdSe:Mn2+ quantum nanoribbons. Nature materials\| PubMed ID: 19915554	2010

Jacek Furdyna

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