femtosecond-laser-filaments-for-use-sub-diffraction-limited-imaging

Femtosecond Laser Filaments for Use in Sub-Diffraction-Limited Imaging and Remote Sensing

Probing remote matter with laser light is a ubiquitous technique used in circumstances as diverse as laser-induced breakdown spectroscopy and barcode ...

Texas A&M University

Baylor University

We develop a technique for optimizing the phase of broad spectrally-separated frequency sidebands-a "holey" spectrum. We use a source of multiple-order coherent Raman sidebands, obtained by crossing femtosecond pump and Stokes beams in synthetic single-crystal diamond. We combine the sidebands into a single beam and show the phase coherence among the sidebands by investigating the interference between them in groups of three while varying one sideband phase by an acousto-optics pulse shaper. We then show how we optimize the broad "holey" spectrum by overcoming the limited temporal shaping window of the pulse shaper. We also explore how the resultant second harmonic/sum frequency generation of the full combined broadband spectrum varies as we vary different sideband phases. This step-by-step phase optimization of the "holey" spectrum can be applied to sidebands with similar structure to synthesize arbitrary optical waveforms.

Shaper-assisted phase optimization of a broad "holey" spectrum.

Achieving super-resolution has become a scientific imperative for remote imaging of objects and scenes needing increased detail and has motivated the development of various laser-based techniques. We demonstrate a scheme which achieves subdiffraction imaging of remote objects by using femtosecond laser filaments. The use of laser filaments for imaging is destined to have applications in many environments.

Remote sub-diffraction imaging with femtosecond laser filaments.

Coherent Anti-Stokes Raman Spectroscopy (CARS) is performed on single spores (conidia) of the fungus Aspergillus nidulans in order to establish a baseline measurement for fungal spores. Chemical maps of single spores are generated and spectral differentiation between the cell wall and the cytoplasm is achieved. Principal Component Analysis of the measured spectra is then completed as a means to quantify spore heterogeneity. Applications range from the quick and accurate diagnosis of public health concerns to real-time agricultural and environmental sensing of fungal symbionts and pathogens.

Article	Year
Shaper-assisted phase optimization of a broad "holey" spectrum. Optics express\| PubMed ID: 22109216	2011
Remote sub-diffraction imaging with femtosecond laser filaments. Optics letters\| PubMed ID: 22513680	2012
CARS spectroscopy of Aspergillus nidulans spores. Scientific reports\| PubMed ID: 30741950	2019

Benjamin D. Strycker

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