The study of the cellular biotransformations of essential or toxic elements requires speciation techniques with high sensitivity and should minimize sample preparation steps that are often prone to modification of chemical species.
Physiological elements such as selenium and iron are known to be particularly difficult to speciate due to their complex chemistry, various stabilities of the selenium or iron species, and their low concentration in the ppm (mg/kg) or even sub-ppm range. Thus, the study of the speciation of these elements by XAS can be extremely challenging. Synchrotron XAS and especially high energy resolution fluorescence detected XAS (HERFD-XAS), which allows a very low signal-to-background ratio1, are available at synchrotron sources to speciate highly diluted elements in complex biological matrices2,3. Conventional fluorescence-XAS measurements can be performed using an energy resolved solid state detector (SSD) with an energy bandwidth ~150–250 eV, on the CRG-FAME beamline at the European Synchrotron Radiation Facility (ESRF)4, while HERFD-XAS measurements need a crystal analyzer spectrometer (CAS), with an energy bandwidth ~1–3 eV, on the CRG-FAME-UHD beamline at the ESRF2. Fluorescence photons are discriminated with respect to their energy with electronic or optical processes respectively.
The sample cryo-preparation is essential to preserve structures and maintain compositional chemical integrity, thus allowing analysis close to the biological native state5. Moreover, analyses performed at cryogenic temperatures as low as 10 K using liquid helium cryogenic cooling (LN2), allow radiation damage to slow down and preserve elemental speciation for XAS. Although some reviews on XAS techniques applied to biological samples report the necessity to prepare and analyze samples in cryogenic conditions (e.g., Sarret et al.6, Porcaro et al.7), none of them clearly describes the related detailed protocol. In this publication, a method for cryo-preparation of cancer cells and plankton microorganisms is described for HERFD-XAS speciation of Se8 and Fe9 at cryogenic temperature.
Good practice for sample preparation and environment during state-of-the-art XAS spectroscopy measurements require 1) a setup; 2) an analysis procedure that limits the effects of radiation damage as much as possible; and 3) a sample (or model compound reference) as homogeneous as possible with respect to the X-ray photons beam size. The first item is taken into account by performing the acquisition at a low temperature, using a liquid helium cryostat. The second item is dealt with by performing each acquisition on a fresh area of the sample by moving it with respect to the beam. Finally, considering the third condition, samples (pellets) and references (powders) are conditioned in pressed bulk pellets in order to limit porosities and inhomogeneities as much as possible, and to avoid roughness with respect to the beam size on the X-ray probed sample surface. We explain how the protocol deals with all of these points.
We used human prostate cell line PC-3 (high metastatic potential) and ovarian cell line OVCAR-3 (which accounts for up to 70% of all ovarian cancer cases) to investigate the antiproliferative properties towards cancer cells of selenium nanoparticles (Se-NPs), and Phaeodactylum tricornutum diatom as a model species to investigate iron sequestration in phytoplankton.